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Catalytic cycle of TYR The catalytic cycle of tyrosinase (Scheme 5) begins with binding of molecular oxygen to the deoxy form of the enzyme (E deoxy , Cu I โCu I ) [139] in the characteristic side-on (ยต-ฮท 2 : ฮท 2 ) binding mode [57] which generates the oxy form (E oxy , Cu II โยต-O 2 โCu II ) that is catalytically competent towards both monophenolic and catecholic substrates [15]
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